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Research Article | Open Access

Light-response adsorption and desorption behaviors of metal–organic frameworks

Chao-Yang Wanga, Lingshan Mab,c, Chong-Chen Wanga( ), Peng Wanga, Leonardo Gutierrezb,c, Weiwei Zhengd
Beijing Key Laboratory of Functional Materials for Building Structure and Environment Remediation/Beijing Energy Conservation & Sustainable Urban and Rural Development Provincial and Ministry Co-construction Collaboration Innovation Center, Beijing University of Civil Engineering and Architecture, Beijing, 100044, PR China
Center for Microbial Ecology and Technology (CMET), Ghent University, Coupure Links 653, 9000, Ghent, Belgium
Center for Advanced Process Technology for Urban Resource Recovery (CAPTURE), Frieda Saeysstraat 1, 9000, Ghent, Belgium
Department of Chemistry, Syracuse University, Syracuse, NY, 13244, United States
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HIGHLIGHTS

• The recent progresses of light-response MOFs were reviewed.

• The light-response adsorption/desorption in aqueous phase were discussed.

• The fabrication strategies of lightresponse MOFs were presented.

• The mechanisms of light-induced adsorption/desorption were summarized.

• The outlooks of the further development of light-response MOFs are proposed.

Abstract

Metal–organic frameworks (MOFs) are ideal adsorbents because of their porous structure, ultra-large specific surface area, abundant active sites, and specific surface charge. Recently, light-response MOFs have received considerable research interests regarding their potential applications in environmental remediation, medical treatment, and artificial intelligence. This review systematically summarizes the recent progress of light-response MOFs and MOF-based composites for light-response adsorption/desorption. The fabrication strategies of light-response MOFs, including in situ synthesis, post-synthesis modification, and introduction of guest molecules, are presented. The mechanisms of light-induced structural change and light-responsive adsorption/desorption are summarized. The prospects for further development of light-response MOFs are discussed. The facile regeneration of light-response MOF-based adsorbents by light irradiation is highly promising for energy saving, environmental friendliness, and sustainability.

Graphical Abstract

Keywords

Light responseMetal–organic frameworksAdsorptionDesorptionMechanism

References

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Environmental Functional Materials
Volume 1 Issue 1,
June 2022
Pages 49-66
DOI: 10.1016/j.efmat.2022.05.002

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Cite this article:
Wang C-Y, Ma L, Wang C-C, et al. Light-response adsorption and desorption behaviors of metal–organic frameworks. Environmental Functional Materials, 2022, 1(1): 49-66. https://doi.org/10.1016/j.efmat.2022.05.002

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Received: 11 April 2022
Revised: 08 May 2022
Accepted: 17 May 2022
Published: 30 May 2022
© 2022 The Authors.

This is an open access article under the CC BY license (http://creativecommons.org/licenses/by/4.0/).